Abstract
(TMTSF)2ClO4 is a quasi-one-dimensional organic conductor and superconductor with Tc=1.4K, and one of at least two Bechgaard salts observed to have upper critical fields far exceeding the paramagnetic limit. Nevertheless, the Se77 NMR Knight shift at low fields reveals a decrease in spin susceptibility χs consistent with singlet spin pairing. The field dependence of the spin-lattice relaxation rate at 100mK exhibits a sharp crossover (or phase transition) at a field Hs∼15kOe, to a regime where χs is close to the normal state value, even though Hc2Hs.
| Original language | English |
|---|---|
| Article number | 147002 |
| Journal | Physical Review Letters |
| Volume | 98 |
| Issue number | 14 |
| Number of pages | 4 |
| ISSN | 0031-9007 |
| DOIs | |
| Publication status | Published - 2007 |
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