Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample

Tetsuya Yokoyama; Meenakshi Wadhwa; Tsuyoshi Iizuka; Vinai Rai; Ikshu Gautam; Yuki Hibiya; Yuki Masuda; Makiko K. Haba; Ryota Fukai; Rebekah Hines; Nicole Phelan; Yoshinari Abe; Jérôme Aléon; Conel M. O'D. Alexander; Sachiko Amari; Yuri Amelin; Ken-ichi Bajo; Martin Bizzarro; Audrey Bouvier; Richard W. Carlson; Marc Chaussidon; Byeon-Gak Choi; Nicolas Dauphas; Andrew M. Davis; Tommaso Di Rocco; Wataru Fujiya; Hiroshi Hidaka; Hisashi Homma; Peter Hoppe; Gary R. Huss; Kiyohiro Ichida; Trevor Ireland; Akira Ishikawa; Shoichi Itoh; Noriyuki Kawasaki; Noriko T. Kita; Koki Kitajima; Thorsten Kleine; Shintaro Komatani; Alexander N. Krot; Ming-Chang Liu; Kevin D. McKeegan; Mayu Morita; Kazuko Motomura; Frédéric Moynier; Izumi Nakai; Kazuhide Nagashima; Ann Nguyen; Larry Nittler; Morihiko Onose; Andreas Pack; Changkun Park; Laurette Piani; Liping Qin; Sara Russell; Naoya Sakamoto; Maria Schönbächler; Lauren Tafla; Haolan Tang; Kentaro Terada; Yasuko Terada; Tomohiro Usui; Sohei Wada; Richard J. Walker; Katsuyuki Yamashita; Qing-Zhu Yin; Shigekazu Yoneda; Edward D. Young; Hiroharu Yui; Ai-Cheng Zhang; Tomoki Nakamura; Hiroshi Naraoka; Takaaki Noguchi; Ryuji Okazaki; Kanako Sakamoto; Hikaru Yabuta; Masanao Abe; Akiko Miyazaki; Aiko Nakato; Masahiro Nishimura; Tatsuaki Okada; Toru Yada; Kasumi Yogata; Satoru Nakazawa; Takanao Saiki; Satoshi Tanaka; Fuyuto Terui; Yuichi Tsuda; Sei-ichiro Watanabe; Makoto Yoshikawa; Shogo Tachibana; Hisayoshi Yurimoto

doi:10.1126/sciadv.adi7048

Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample

Tetsuya Yokoyama^*, Meenakshi Wadhwa, Tsuyoshi Iizuka, Vinai Rai, Ikshu Gautam, Yuki Hibiya, Yuki Masuda, Makiko K. Haba, Ryota Fukai, Rebekah Hines, Nicole Phelan, Yoshinari Abe, Jérôme Aléon, Conel M. O'D. Alexander, Sachiko Amari, Yuri Amelin, Ken-ichi Bajo, Martin Bizzarro, Audrey Bouvier, Richard W. CarlsonMarc Chaussidon, Byeon-Gak Choi, Nicolas Dauphas, Andrew M. Davis, Tommaso Di Rocco, Wataru Fujiya, Hiroshi Hidaka, Hisashi Homma, Peter Hoppe, Gary R. Huss, Kiyohiro Ichida, Trevor Ireland, Akira Ishikawa, Shoichi Itoh, Noriyuki Kawasaki, Noriko T. Kita, Koki Kitajima, Thorsten Kleine, Shintaro Komatani, Alexander N. Krot, Ming-Chang Liu, Kevin D. McKeegan, Mayu Morita, Kazuko Motomura, Frédéric Moynier, Izumi Nakai, Kazuhide Nagashima, Ann Nguyen, Larry Nittler, Morihiko Onose, Andreas Pack, Changkun Park, Laurette Piani, Liping Qin, Sara Russell, Naoya Sakamoto, Maria Schönbächler, Lauren Tafla, Haolan Tang, Kentaro Terada, Yasuko Terada, Tomohiro Usui, Sohei Wada, Richard J. Walker, Katsuyuki Yamashita, Qing-Zhu Yin, Shigekazu Yoneda, Edward D. Young, Hiroharu Yui, Ai-Cheng Zhang, Tomoki Nakamura, Hiroshi Naraoka, Takaaki Noguchi, Ryuji Okazaki, Kanako Sakamoto, Hikaru Yabuta, Masanao Abe, Akiko Miyazaki, Aiko Nakato, Masahiro Nishimura, Tatsuaki Okada, Toru Yada, Kasumi Yogata, Satoru Nakazawa, Takanao Saiki, Satoshi Tanaka, Fuyuto Terui, Yuichi Tsuda, Sei-ichiro Watanabe, Makoto Yoshikawa, Shogo Tachibana, Hisayoshi Yurimoto

^*Corresponding author for this work

Centre for Star and Planet Formation

Research output: Contribution to journal › Journal article › Research › peer-review

14 Citations (Scopus)

6 Downloads (Pure)

Abstract

Studies of material returned from Cb asteroid Ryugu have revealed considerable mineralogical and chemical heterogeneity, stemming primarily from brecciation and aqueous alteration. Isotopic anomalies could have also been affected by delivery of exogenous clasts and aqueous mobilization of soluble elements. Here, we show that isotopic anomalies for mildly soluble Cr are highly variable in Ryugu and CI chondrites, whereas those of Ti are relatively uniform. This variation in Cr isotope ratios is most likely due to physicochemical fractionation between ⁵⁴Cr-rich presolar nanoparticles and Cr-bearing secondary minerals at the millimeter-scale in the bulk samples, likely due to extensive aqueous alteration in their parent bodies that occurred 5:2^þ1₁^:_:⁸₄ Ma after Solar System birth. In contrast, Ti isotopes were marginally affected by this process. Our results show that isotopic heterogeneities in asteroids are not all nebular or accretionary in nature but can also reflect element redistribution by water.

Original language	English
Article number	eadi7048
Journal	Science Advances
Volume	9
Issue number	45
Number of pages	11
ISSN	2375-2548
DOIs	https://doi.org/10.1126/sciadv.adi7048
Publication status	Published - 2023

Bibliographical note

Publisher Copyright:
© 2023 American Association for the Advancement of Science. All rights reserved.

Access to Document

10.1126/sciadv.adi7048Licence: CC BY-NC

FulltextFinal published version, 1.07 MBLicence: CC BY-NC

Cite this

Yokoyama, T., Wadhwa, M., Iizuka, T., Rai, V., Gautam, I., Hibiya, Y., Masuda, Y., Haba, M. K., Fukai, R., Hines, R., Phelan, N., Abe, Y., Aléon, J., Alexander, C. M. OD., Amari, S., Amelin, Y., Bajo, K., Bizzarro, M., Bouvier, A., ... Yurimoto, H. (2023). Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample. Science Advances, 9(45), [eadi7048]. https://doi.org/10.1126/sciadv.adi7048

Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample. / Yokoyama, Tetsuya; Wadhwa, Meenakshi; Iizuka, Tsuyoshi; Rai, Vinai; Gautam, Ikshu; Hibiya, Yuki; Masuda, Yuki; Haba, Makiko K.; Fukai, Ryota; Hines, Rebekah; Phelan, Nicole; Abe, Yoshinari; Aléon, Jérôme; Alexander, Conel M. O'D.; Amari, Sachiko; Amelin, Yuri; Bajo, Ken-ichi; Bizzarro, Martin; Bouvier, Audrey; Carlson, Richard W.; Chaussidon, Marc; Choi, Byeon-Gak; Dauphas, Nicolas; Davis, Andrew M.; Rocco, Tommaso Di; Fujiya, Wataru; Hidaka, Hiroshi; Homma, Hisashi; Hoppe, Peter; Huss, Gary R.; Ichida, Kiyohiro; Ireland, Trevor; Ishikawa, Akira; Itoh, Shoichi; Kawasaki, Noriyuki; Kita, Noriko T.; Kitajima, Koki; Kleine, Thorsten; Komatani, Shintaro; Krot, Alexander N.; Liu, Ming-Chang; McKeegan, Kevin D.; Morita, Mayu; Motomura, Kazuko; Moynier, Frédéric; Nakai, Izumi; Nagashima, Kazuhide; Nguyen, Ann; Nittler, Larry; Onose, Morihiko; Pack, Andreas; Park, Changkun; Piani, Laurette; Qin, Liping; Russell, Sara; Sakamoto, Naoya; Schönbächler, Maria; Tafla, Lauren; Tang, Haolan; Terada, Kentaro; Terada, Yasuko; Usui, Tomohiro; Wada, Sohei; Walker, Richard J.; Yamashita, Katsuyuki; Yin, Qing-Zhu; Yoneda, Shigekazu; Young, Edward D.; Yui, Hiroharu; Zhang, Ai-Cheng; Nakamura, Tomoki; Naraoka, Hiroshi; Noguchi, Takaaki; Okazaki, Ryuji; Sakamoto, Kanako; Yabuta, Hikaru; Abe, Masanao; Miyazaki, Akiko; Nakato, Aiko; Nishimura, Masahiro; Okada, Tatsuaki; Yada, Toru; Yogata, Kasumi; Nakazawa, Satoru; Saiki, Takanao; Tanaka, Satoshi; Terui, Fuyuto; Tsuda, Yuichi; Watanabe, Sei-ichiro; Yoshikawa, Makoto; Tachibana, Shogo; Yurimoto, Hisayoshi.

In: Science Advances, Vol. 9, No. 45, eadi7048, 2023.

Research output: Contribution to journal › Journal article › Research › peer-review

Yokoyama, T, Wadhwa, M, Iizuka, T, Rai, V, Gautam, I, Hibiya, Y, Masuda, Y, Haba, MK, Fukai, R, Hines, R, Phelan, N, Abe, Y, Aléon, J, Alexander, CMOD, Amari, S, Amelin, Y, Bajo, K, Bizzarro, M, Bouvier, A, Carlson, RW, Chaussidon, M, Choi, B-G, Dauphas, N, Davis, AM, Rocco, TD, Fujiya, W, Hidaka, H, Homma, H, Hoppe, P, Huss, GR, Ichida, K, Ireland, T, Ishikawa, A, Itoh, S, Kawasaki, N, Kita, NT, Kitajima, K, Kleine, T, Komatani, S, Krot, AN, Liu, M-C, McKeegan, KD, Morita, M, Motomura, K, Moynier, F, Nakai, I, Nagashima, K, Nguyen, A, Nittler, L, Onose, M, Pack, A, Park, C, Piani, L, Qin, L, Russell, S, Sakamoto, N, Schönbächler, M, Tafla, L, Tang, H, Terada, K, Terada, Y, Usui, T, Wada, S, Walker, RJ, Yamashita, K, Yin, Q-Z, Yoneda, S, Young, ED, Yui, H, Zhang, A-C, Nakamura, T, Naraoka, H, Noguchi, T, Okazaki, R, Sakamoto, K, Yabuta, H, Abe, M, Miyazaki, A, Nakato, A, Nishimura, M, Okada, T, Yada, T, Yogata, K, Nakazawa, S, Saiki, T, Tanaka, S, Terui, F, Tsuda, Y, Watanabe, S, Yoshikawa, M, Tachibana, S & Yurimoto, H 2023, 'Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample', Science Advances, vol. 9, no. 45, eadi7048. https://doi.org/10.1126/sciadv.adi7048

Yokoyama, Tetsuya ; Wadhwa, Meenakshi ; Iizuka, Tsuyoshi ; Rai, Vinai ; Gautam, Ikshu ; Hibiya, Yuki ; Masuda, Yuki ; Haba, Makiko K. ; Fukai, Ryota ; Hines, Rebekah ; Phelan, Nicole ; Abe, Yoshinari ; Aléon, Jérôme ; Alexander, Conel M. O'D. ; Amari, Sachiko ; Amelin, Yuri ; Bajo, Ken-ichi ; Bizzarro, Martin ; Bouvier, Audrey ; Carlson, Richard W. ; Chaussidon, Marc ; Choi, Byeon-Gak ; Dauphas, Nicolas ; Davis, Andrew M. ; Rocco, Tommaso Di ; Fujiya, Wataru ; Hidaka, Hiroshi ; Homma, Hisashi ; Hoppe, Peter ; Huss, Gary R. ; Ichida, Kiyohiro ; Ireland, Trevor ; Ishikawa, Akira ; Itoh, Shoichi ; Kawasaki, Noriyuki ; Kita, Noriko T. ; Kitajima, Koki ; Kleine, Thorsten ; Komatani, Shintaro ; Krot, Alexander N. ; Liu, Ming-Chang ; McKeegan, Kevin D. ; Morita, Mayu ; Motomura, Kazuko ; Moynier, Frédéric ; Nakai, Izumi ; Nagashima, Kazuhide ; Nguyen, Ann ; Nittler, Larry ; Onose, Morihiko ; Pack, Andreas ; Park, Changkun ; Piani, Laurette ; Qin, Liping ; Russell, Sara ; Sakamoto, Naoya ; Schönbächler, Maria ; Tafla, Lauren ; Tang, Haolan ; Terada, Kentaro ; Terada, Yasuko ; Usui, Tomohiro ; Wada, Sohei ; Walker, Richard J. ; Yamashita, Katsuyuki ; Yin, Qing-Zhu ; Yoneda, Shigekazu ; Young, Edward D. ; Yui, Hiroharu ; Zhang, Ai-Cheng ; Nakamura, Tomoki ; Naraoka, Hiroshi ; Noguchi, Takaaki ; Okazaki, Ryuji ; Sakamoto, Kanako ; Yabuta, Hikaru ; Abe, Masanao ; Miyazaki, Akiko ; Nakato, Aiko ; Nishimura, Masahiro ; Okada, Tatsuaki ; Yada, Toru ; Yogata, Kasumi ; Nakazawa, Satoru ; Saiki, Takanao ; Tanaka, Satoshi ; Terui, Fuyuto ; Tsuda, Yuichi ; Watanabe, Sei-ichiro ; Yoshikawa, Makoto ; Tachibana, Shogo ; Yurimoto, Hisayoshi. / Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample. In: Science Advances. 2023 ; Vol. 9, No. 45.

@article{09ad3f2290d14ca8a6403386e80b8470,

title = "Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample",

abstract = "Studies of material returned from Cb asteroid Ryugu have revealed considerable mineralogical and chemical heterogeneity, stemming primarily from brecciation and aqueous alteration. Isotopic anomalies could have also been affected by delivery of exogenous clasts and aqueous mobilization of soluble elements. Here, we show that isotopic anomalies for mildly soluble Cr are highly variable in Ryugu and CI chondrites, whereas those of Ti are relatively uniform. This variation in Cr isotope ratios is most likely due to physicochemical fractionation between 54Cr-rich presolar nanoparticles and Cr-bearing secondary minerals at the millimeter-scale in the bulk samples, likely due to extensive aqueous alteration in their parent bodies that occurred 5:2{\th}11::84 Ma after Solar System birth. In contrast, Ti isotopes were marginally affected by this process. Our results show that isotopic heterogeneities in asteroids are not all nebular or accretionary in nature but can also reflect element redistribution by water.",

author = "Tetsuya Yokoyama and Meenakshi Wadhwa and Tsuyoshi Iizuka and Vinai Rai and Ikshu Gautam and Yuki Hibiya and Yuki Masuda and Haba, {Makiko K.} and Ryota Fukai and Rebekah Hines and Nicole Phelan and Yoshinari Abe and J{\'e}r{\^o}me Al{\'e}on and Alexander, {Conel M. O'D.} and Sachiko Amari and Yuri Amelin and Ken-ichi Bajo and Martin Bizzarro and Audrey Bouvier and Carlson, {Richard W.} and Marc Chaussidon and Byeon-Gak Choi and Nicolas Dauphas and Davis, {Andrew M.} and Rocco, {Tommaso Di} and Wataru Fujiya and Hiroshi Hidaka and Hisashi Homma and Peter Hoppe and Huss, {Gary R.} and Kiyohiro Ichida and Trevor Ireland and Akira Ishikawa and Shoichi Itoh and Noriyuki Kawasaki and Kita, {Noriko T.} and Koki Kitajima and Thorsten Kleine and Shintaro Komatani and Krot, {Alexander N.} and Ming-Chang Liu and McKeegan, {Kevin D.} and Mayu Morita and Kazuko Motomura and Fr{\'e}d{\'e}ric Moynier and Izumi Nakai and Kazuhide Nagashima and Ann Nguyen and Larry Nittler and Morihiko Onose and Andreas Pack and Changkun Park and Laurette Piani and Liping Qin and Sara Russell and Naoya Sakamoto and Maria Sch{\"o}nb{\"a}chler and Lauren Tafla and Haolan Tang and Kentaro Terada and Yasuko Terada and Tomohiro Usui and Sohei Wada and Walker, {Richard J.} and Katsuyuki Yamashita and Qing-Zhu Yin and Shigekazu Yoneda and Young, {Edward D.} and Hiroharu Yui and Ai-Cheng Zhang and Tomoki Nakamura and Hiroshi Naraoka and Takaaki Noguchi and Ryuji Okazaki and Kanako Sakamoto and Hikaru Yabuta and Masanao Abe and Akiko Miyazaki and Aiko Nakato and Masahiro Nishimura and Tatsuaki Okada and Toru Yada and Kasumi Yogata and Satoru Nakazawa and Takanao Saiki and Satoshi Tanaka and Fuyuto Terui and Yuichi Tsuda and Sei-ichiro Watanabe and Makoto Yoshikawa and Shogo Tachibana and Hisayoshi Yurimoto",

year = "2023",

doi = "10.1126/sciadv.adi7048",

language = "English",

volume = "9",

journal = "Science advances",

issn = "2375-2548",

publisher = "American Association for the Advancement of Science",

number = "45",

}

TY - JOUR

T1 - Water circulation in Ryugu asteroid affected the distribution of nucleosynthetic isotope anomalies in returned sample

AU - Yokoyama, Tetsuya

AU - Wadhwa, Meenakshi

AU - Iizuka, Tsuyoshi

AU - Rai, Vinai

AU - Gautam, Ikshu

AU - Hibiya, Yuki

AU - Masuda, Yuki

AU - Haba, Makiko K.

AU - Fukai, Ryota

AU - Hines, Rebekah

AU - Phelan, Nicole

AU - Abe, Yoshinari

AU - Aléon, Jérôme

AU - Alexander, Conel M. O'D.

AU - Amari, Sachiko

AU - Amelin, Yuri

AU - Bajo, Ken-ichi

AU - Bizzarro, Martin

AU - Bouvier, Audrey

AU - Carlson, Richard W.

AU - Chaussidon, Marc

AU - Choi, Byeon-Gak

AU - Dauphas, Nicolas

AU - Davis, Andrew M.

AU - Rocco, Tommaso Di

AU - Fujiya, Wataru

AU - Hidaka, Hiroshi

AU - Homma, Hisashi

AU - Hoppe, Peter

AU - Huss, Gary R.

AU - Ichida, Kiyohiro

AU - Ireland, Trevor

AU - Ishikawa, Akira

AU - Itoh, Shoichi

AU - Kawasaki, Noriyuki

AU - Kita, Noriko T.

AU - Kitajima, Koki

AU - Kleine, Thorsten

AU - Komatani, Shintaro

AU - Krot, Alexander N.

AU - Liu, Ming-Chang

AU - McKeegan, Kevin D.

AU - Morita, Mayu

AU - Motomura, Kazuko

AU - Moynier, Frédéric

AU - Nakai, Izumi

AU - Nagashima, Kazuhide

AU - Nguyen, Ann

AU - Nittler, Larry

AU - Onose, Morihiko

AU - Pack, Andreas

AU - Park, Changkun

AU - Piani, Laurette

AU - Qin, Liping

AU - Russell, Sara

AU - Sakamoto, Naoya

AU - Schönbächler, Maria

AU - Tafla, Lauren

AU - Tang, Haolan

AU - Terada, Kentaro

AU - Terada, Yasuko

AU - Usui, Tomohiro

AU - Wada, Sohei

AU - Walker, Richard J.

AU - Yamashita, Katsuyuki

AU - Yin, Qing-Zhu

AU - Yoneda, Shigekazu

AU - Young, Edward D.

AU - Yui, Hiroharu

AU - Zhang, Ai-Cheng

AU - Nakamura, Tomoki

AU - Naraoka, Hiroshi

AU - Noguchi, Takaaki

AU - Okazaki, Ryuji

AU - Sakamoto, Kanako

AU - Yabuta, Hikaru

AU - Abe, Masanao

AU - Miyazaki, Akiko

AU - Nakato, Aiko

AU - Nishimura, Masahiro

AU - Okada, Tatsuaki

AU - Yada, Toru

AU - Yogata, Kasumi

AU - Nakazawa, Satoru

AU - Saiki, Takanao

AU - Tanaka, Satoshi

AU - Terui, Fuyuto

AU - Tsuda, Yuichi

AU - Watanabe, Sei-ichiro

AU - Yoshikawa, Makoto

AU - Tachibana, Shogo

AU - Yurimoto, Hisayoshi

PY - 2023

Y1 - 2023

N2 - Studies of material returned from Cb asteroid Ryugu have revealed considerable mineralogical and chemical heterogeneity, stemming primarily from brecciation and aqueous alteration. Isotopic anomalies could have also been affected by delivery of exogenous clasts and aqueous mobilization of soluble elements. Here, we show that isotopic anomalies for mildly soluble Cr are highly variable in Ryugu and CI chondrites, whereas those of Ti are relatively uniform. This variation in Cr isotope ratios is most likely due to physicochemical fractionation between 54Cr-rich presolar nanoparticles and Cr-bearing secondary minerals at the millimeter-scale in the bulk samples, likely due to extensive aqueous alteration in their parent bodies that occurred 5:2þ11::84 Ma after Solar System birth. In contrast, Ti isotopes were marginally affected by this process. Our results show that isotopic heterogeneities in asteroids are not all nebular or accretionary in nature but can also reflect element redistribution by water.

AB - Studies of material returned from Cb asteroid Ryugu have revealed considerable mineralogical and chemical heterogeneity, stemming primarily from brecciation and aqueous alteration. Isotopic anomalies could have also been affected by delivery of exogenous clasts and aqueous mobilization of soluble elements. Here, we show that isotopic anomalies for mildly soluble Cr are highly variable in Ryugu and CI chondrites, whereas those of Ti are relatively uniform. This variation in Cr isotope ratios is most likely due to physicochemical fractionation between 54Cr-rich presolar nanoparticles and Cr-bearing secondary minerals at the millimeter-scale in the bulk samples, likely due to extensive aqueous alteration in their parent bodies that occurred 5:2þ11::84 Ma after Solar System birth. In contrast, Ti isotopes were marginally affected by this process. Our results show that isotopic heterogeneities in asteroids are not all nebular or accretionary in nature but can also reflect element redistribution by water.

U2 - 10.1126/sciadv.adi7048

DO - 10.1126/sciadv.adi7048

M3 - Journal article

C2 - 37939187

AN - SCOPUS:85181047049

VL - 9

JO - Science advances

JF - Science advances

SN - 2375-2548

IS - 45

M1 - eadi7048

ER -